In this comprehensive review, a systematic overview of progress in inhibition methods of HER is provided, including anodic alloying, structural treatment, surface modification, additives and non-aq.
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What''s worse, the defects and GBs provide pathways for ion migration. Therefore, future endeavor could involve the fabrication of perovskite single-crystal solar cells, in which perovskite single crystals are free of GBs and have significantly low defect densities.
There is no doubt that the investigation of ion migration and the summarization of recent advances in inhibition strategies are necessary to develop "state-of-the-art" PVSCs with high intrinsic stability for accelerated
With an excellent power conversion efficiency of 25.7%, closer to the Shockley–Queisser limit, perovskite solar cells (PSCs) have become a strong candidate for a next-generation energy harvester. However, the lack of stability and reliability in PSCs remained challenging for commercialization. Strategies, such as interfacial and structural engineering,
Overall, it was found that hydrogen can deactivate most of typical defects (sometimes induce defect) in n- and p-type crystalline silicon, leading to a significant efficiency enhancement in passivated emitter rear contact, TOPCon and SHJ solar cells.
Hydrogen evolution reaction (HER) and sulfation on the negative plate are main problems hindering the operation of lead-carbon batteries under high-rate partial-state-of
Interface-induced nonradiative recombination losses at the perovskite/electron transport layer (ETL) are an impediment to improving the efficiency and stability of inverted (p-i-n) perovskite solar cells (PSCs). Tridecafluorohexane-1-sulfonic acid potassium (TFHSP) is employed as a multifunctional dipole molecule to modify the perovskite
To improve the understanding of hydrogen in silicon solar cells, measurement techniques such as vibrational spectroscopy, ECV, and nuclear resonance reaction analysis have been used to establish direct correlations with hydrogen passivation reactions, providing strong evidence of the involvement of hydrogen for example in the passivation of
The quest for efficient green hydrogen production through Alkaline Water Electrolysis (AWE) is a critical aspect of the clean energy transition. The hydrogen evolution reaction (HER) in alkaline media is central to this process, with the performance of electrocatalysts being a determining factor for overall efficiency. Theoretical studies using
Intrinsic ion migration in the metal halide perovskite (MHP) absorber layer and its interfaces seriously limits the device stability of perovskite solar cells (PSCs). Despite considerable efforts to mitigate the ion migration issue, it remains a formidable challenge in the commercialization of PSCs. Here, we provide a short review of the device failure mechanisms
We discover that the chemical potential for mobile hydrogen develops a gradient, forcing the hydrogen to drift from the interface, leaving behind recombination-active
1 天前· Inverted-pyramid black silicon photocathodes were prepared using Cu-MACE for solar hydrogen evolution. TMAH optimization identified the surface structure for the best PEC
The in situ formation of methyl tetrahydrotriazinium (MTTZ+) and dimethylammonium cations improves film crystallinity in perovskite solar cells.
Overall, it was found that hydrogen can deactivate most of typical defects (sometimes induce defect) in n- and p-type crystalline silicon, leading to a significant efficiency
In this study, a novel sulfamic acid-caprolactam based electrolytes for inhibiting hydrogen evolution in the proton batteries was investigated. Aminosulfonic acid was used as a proton source in the proton batteries for the first time. In addition, caprolactam cosolvent with double hydrogen bond site was added to the electrolyte to help H
Here, we summarize the hydrogen bonding in PSCs, including each functional layer and interface. Despite being a weak force, hydrogen bonding can greatly influence material properties. Effects and strategies to precisely adjust hydrogen bonding for
In this study, a novel sulfamic acid-caprolactam based electrolytes for inhibiting hydrogen evolution in the proton batteries was investigated. Aminosulfonic acid was used as a
There is no doubt that the investigation of ion migration and the summarization of recent advances in inhibition strategies are necessary to develop "state-of-the-art" PVSCs with high intrinsic stability for accelerated commercialization.
Driving the electrocatalytic hydrogen evolution reaction (HER) with solar-energy cells is considered a green and sustainable way to produce H2. Herein, CoO-Mo2N hollow heterojunctions were
1 天前· Inverted-pyramid black silicon photocathodes were prepared using Cu-MACE for solar hydrogen evolution. TMAH optimization identified the surface structure for the best PEC performance. In situ construction of PN junctions reduced the hydrogen evolution external bias.
To improve the understanding of hydrogen in silicon solar cells, measurement techniques such as vibrational spectroscopy, ECV, and nuclear resonance reaction analysis have been used to establish direct correlations with
Perovskite solar cells have made significant strides in recent years. However, there are still challenges in terms of photoelectric conversion efficiency and long-term stability associated with perovskite solar cells. The presence of defects in perovskite materials is one of the important influencing factors leading to subpar film quality. Adopting additives to passivate
Three polymer acceptors named PTz-Ph, PTz-Me, and PTz-H are synthesized by substituting the Phenyl, Methyl, and Hydrogen in the beta position of the thiophene unit based on small molecules. PTz-H-based device achieves a record-high efficiency of 18.16% and the highest photocurrent for all-polymer solar cells reported in the literature thus far.
Semantic Scholar extracted view of "Strong Hydrogen-Bonded Interfacial Water Inhibiting Hydrogen Evolution Kinetics to Promote Electrochemical CO2 Reduction to C2+" by Yang Wang et al. Skip to search form Skip to main content Skip to account menu. Semantic Scholar''s Logo. Search 223,176,311 papers from all fields of science. Search. Sign In Create
Hydrogen evolution reaction (HER) and sulfation on the negative plate are main problems hindering the operation of lead-carbon batteries under high-rate partial-state-of-charge (HRPSoC). Here, reduced graphene oxide nanosheets modified with graphitic carbon nitride (g-C 3 N 4 @rGO) were prepared and used as additives in an attempt to solve the
We discover that the chemical potential for mobile hydrogen develops a gradient, forcing the hydrogen to drift from the interface, leaving behind recombination-active defects. We find...
Interface-induced nonradiative recombination losses at the perovskite/electron transport layer (ETL) are an impediment to improving the efficiency and stability of inverted (p-i-n) perovskite solar cells (PSCs). Tridecafluorohexane-1-sulfonic acid potassium (TFHSP) is
Inhibiting Interfacial Nonradiative Recombination in Inverted Perovskite Solar Cells with a Multifunctional Molecule. The solid coordination and hydrogen bonding efficiently passivate the surface defects, thereby reducing nonradiative recombination. The induced positive dipole layer between the perovskite and ETLs improves the energy band alignment, enhancing
Here, we summarize the hydrogen bonding in PSCs, including each functional layer and interface. Despite being a weak force, hydrogen bonding can greatly influence material properties. Effects and strategies to
Polymerization of Y6-type acceptor molecules leads to bulk-heterojunction organic solar cells with both high power-conversion efficiency and device stability, but the underlying mechanism remains
This is largely due to the complex behaviour of hydrogen in silicon and its ability to exist in many different forms in the lattice. For commercial solar cells, hydrogen is introduced into the device through the deposition of hydrogen-containing dielectric layers and the subsequent metallisation firing process.
With the implementation of such processes for industrial silicon solar cells, efficiency improvements of 1.1% absolute can be obtained. Hydrogen passivation is widely used for silicon solar cells to reduce the recombination activity associated with a variety of performance limiting defects.
P-type monocrystalline silicon solar cells receive benefits of hydrogen passivation of metastable defects such as the carrier-induced boron-oxygen (B-O) defect. [36, 37] B-O defects can form under the normal operating conditions in the field, causing a reduction in cell performance of up to 2% absolute.
A key defect in silicon solar cells plagued with contradictions is the B-O complex. In particular, controversy has surrounded the role of hydrogen in the permanent deactivation process.
However, caution should be taken as excess interstitial hydrogen can also cause a range of detrimental effects in silicon solar cells such as the formation of recombination active hydrogen-defect complexes, LeTID, and contact resistance issues.
If the analysis in this paper is correct, then the paper by Walter et al provides an excellent example where, even when trying to avoid hydrogen incorporation in a silicon solar cell, hydrogen can still be present in the wafer and can therefore influence an experiment.
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